- Antonio Clareti Pereira, PhD
- PhD in Chemical Engineering University of São Paulo (USP) Belo Horizonte, Minas Gerais, Brazil
- DOI: 10.5281/zenodo.21862522
Gallium recovery from zinc-processing residues has
expanded rapidly, yet the evidence remains heterogeneous and heavily weighted
toward laboratory studies. This structured critical narrative review examines
95 publications issued from January 2020 to July 2026 on gallium deportment,
residue formation, characterization, pretreatment, leaching, purification,
separation, and product recovery in zinc metallurgical residues and integrated
Zn–Pb materials. The corpus was assembled using reproducible keyword
combinations, DOI- and title-based deduplication, single-reviewer screening,
and study-level evidence coding. Seventy-three empirical or mechanistic
publications were graded by evidence type (A = 4, B = 8, C = 20, D = 22, and E
= 19), while 22 review, contextual, thesis, or proceedings publications were
retained as supporting evidence; only a small minority used continuous, factory,
or industrially representative operations. Quantitative comparisons show that
host-phase control is decisive: industrial optimization increased gallium
leaching from 77.83% to 96.46% when jarosite-associated gallium was addressed,
while selected downstream operations achieved 97.9% iron removal before gallium
extraction, up to 99% gallium recovery in staged membrane contact, and 98.6%
adsorption after six resin cycles. Zinc-refinery and replacement residues
provide the strongest evidence. Data for primary lead residues remain
insufficient and are therefore treated as complementary evidence from
integrated Zn–Pb materials rather than as an equivalent evidence base.
High-confidence conclusions concern the importance of mineral hosting, iron
control, complete mass balance, and multimetal integration. Claims regarding
universal flowsheets, economic thresholds, and industrial circularity remain
low confidence because continuous campaigns, reagent recycle, product
qualification, and comparable techno-economic or life-cycle data are scarce.

